The outlet, which will open at Bond Street this week, follows a debut at London's Liverpool Street station last November.
The company is attempting to build the first UK chain of iPod-dedicated shops and the intention is to have 12 UK stores by the end of the year.
The shop will occupy two floors and features a minimalist design in keeping with the Apple aesthetic. Stores carry a full range of iPod products and a vast array of accessories.
PopXpress is also selling own-brand products, including leather cases, headphones, adaptors and even iPod-enabled boxer shorts.
PopXpress chief executive Jonathan Cole said: 'After the success of the first store at Liverpool Street, we are thrilled to be opening this second store in such a prestigious retail district, at such an exciting time in the iPod's development.'
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