Foyles will join Marks & Spencer, a daily farmers' market and various restaurants and bars in the Eurostar terminus. The cross-channel train terminus will move from Waterloo to the St Pancras in November.
The Victorian station has undergone a 10-year£800 million restoration and regeneration project.
Foyles will stock about 20,000 titles, including foreign language books, in the 3,040 sq ft (280 sq m) store.
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