The outlet can be found in the sound and vision department on the third floor and stocks the full range of handsets and accessories.
Vodafone UK head of retail Tom Devine said: 'This is an exciting time for Vodafone to be working with Harrods and has already proved to be a successful venture during the short time that the store has been trading.
'Brompton Road has always been a specific target location for Vodafone in order to be accessible to Knightsbridge shoppers. We're pleased to offer Christmas shoppers in Harrods the latest mobiles and tariffs from Vodafone.'
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