Jovovich, who is famed for her role in the film Fifth Element, is signed to the deal until December. The actress is also an accomplished fashion designer and has her own brand, Jovovich-Hawk.
The high street retailer unveiled the campaign at its Oxford Street store today.
Mango is the latest in a raft of high street retailers, including Goldsmiths and Monsoon, to reveal celebrity-endorsed campaigns in recent weeks.
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